...do the different mixes of SMART attributes reported for my Samsung and SanDisk SSDs give either report an edge in assisting me in anticipating drive failure?
Yes — if you understand enough about what they are reporting to interpret the attributes. There are a whole series of SMART attributes for hard drives and SATA connected SSDs that are intended to indicate a drive is in a "pre-failure" status, and others that indicate the age of the drive and both are so designated in the Drive Scope report. Whether a report indicates a parameter is a "pre-fail" indicator or not that attribute still indicates "pre-fail status". See
Drive Scope HD Attributes. Any positive number in a pre-fail attribute is at least a caution flag. If a pre-fail attribute racks up half of the threshold value you should have the drives replacement on order and planning your switchover strategy. Typically the closer you get to a threshold value the faster the rate of deteriration.